Improved neural networks for the classification of microplastics via inferior quality Raman spectra.

Journal: Talanta
Published Date:

Abstract

Machine learning algorithms are proficient in the rapid extraction of features for the classification of microplastic Raman spectra. Nevertheless, the classification of Raman spectra from microplastics, particularly in the presence of complex environmental interference, remains a substantial challenge. In this study, an improved ResNet model incorporating the Squeeze-and-Excitation (SE) module is employed for the classification and identification of Raman spectra of microplastics across varying quality levels under diverse experimental conditions with insufficient laser power and short spectrum acquisition time. The improved ResNet model exhibits superior accuracy in classifying inferior quality Raman spectra characterized by significant noise and low signal-to-noise ratios, as compared to traditional CNN, without a considerable escalation in parameter size or computational burden. Even under the most adverse experimental conditions assessed, the model achieved a notable recognition accuracy of 97.83 %. Moreover, the application of Grad-CAM visualization provides insights into the criteria underlying machine learning-based spectral classification. This research underscores the capacity of machine learning algorithms in the analysis and interpretation of inferior quality Raman spectra within complex and non-ideal experimental scenarios.

Authors

  • Weixiang Huang
    School of Environmental Science and Optoelectronic Technology, University of Science and Technology of China, Hefei, 230026, China; Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, 230031, China.
  • Jiajin Chen
    Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, 230031, China. Electronic address: jjchen@aiofm.ac.cn.
  • Hao Xiong
  • Tu Tan
    Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, 230031, China.
  • Guishi Wang
    Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, Anhui 230037, China.
  • Kun Liu
    Department of Anesthesiology, Shanghai Chest Hospital, Shanghai Jiao Tong University, Shanghai 200030, China.
  • Chilai Chen
    Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, 230031, China.
  • Xiaoming Gao
    College of Environmental Science and Optoelectronic Technology, University of Science and Technology of China, Hefei, Anhui 230026, China.

Keywords

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