Machine learning based prediction of mechanical properties in carbon fiber recovered through pyrolysis.

Journal: Waste management (New York, N.Y.)
Published Date:

Abstract

The limitations of traditional pyrolysis technologies of recovered carbon fiber included long processing time, low efficiency, and unclear links between process parameters and performance. Moreover, pyrolysis alone formed residual coke on carbon fiber surfaces, severely impairing reusability. Therefore, this study adopted a combination of pyrolysis oxidation recycling to obtain clean carbon fibers, and introduced an innovative machine learning optimization framework to predict and analyze key recycling parameters. Specifically, a database of raw material characteristics and process parameters was built via systematic literature research. Subsequently, four machine learning models were integrated to predict mechanical performance, and the random forest model performed the best with determination coefficients of 0.9608 and 0.9419, respectively. Additionally, partial dependency graph analysis quantified the process window and determined the optimal parameters. Optimal tensile modulus was attained with a 5 ℃/min pyrolysis rate, 570 ℃ oxidation temperature, and 45%-75% carbon fiber mass fraction. For tensile strength, the best parameters were 557 ℃ oxidation temperature and 45 mins oxidation time. A 5 ℃/min pyrolysis rate stabilized tensile modulus, while 500 ℃ preserved tensile strength. Additionally, 75 wt% carbon content combined with high fiber mass fraction enhanced mechanical performance. The foundation was laid for subsequent pyrolysis‑oxidation experiments on carbon‑fiber recovery, and the recovery efficiency was improved. Overall, this study can provide more accurate theoretical support for carbon fiber recycling technology.

Authors

  • Xiang Guo
    State Key Laboratory of Oncology in South China, Collaborative Innovation Center of Cancer Medicine, Guangzhou, 510060, P. R. China. [email protected].
  • Tian Li
    College of Plant Protection, Southwest University, Chongqing, China.
  • Chunting Liu
    School of Transportation Science and Engineering, Civil Aviation University of China, Tianjin 300300, China.
  • Meng Zhang
    College of Software, Beihang University, Beijing, China.
  • Hao Li
    Department of Urology, Tongji Hospital, Tongji Medical College, Huazhong University of Science and Technology, Wuhan, China.
  • Jinrui Li
    School of Transportation Science and Engineering, Civil Aviation University of China, Tianjin 300300, China.
  • Yihua Zhang
    Library, Chengdu University of Information Technology, Chengdu 610225, China.
  • Chunmei Zeng
    School of Transportation Science and Engineering, Civil Aviation University of China, Tianjin 300300, China.
  • Shuwu Wei
    College of Engineering, Zhejiang Normal University, Jinhua, China.
  • Linlin Pei
    School of Transportation Science and Engineering, Civil Aviation University of China, Tianjin 300300, China.
  • Fang Liu
    The First Clinical Medical College of Gannan Medical University, Ganzhou 341000, Jiangxi Province, China.
  • Da Chen
    College of Electronics and Information Engineering, Shandong University of Science and Technology, Qingdao, China.

Keywords

No keywords available for this article.