A robust black carbon prediction model derived from observational datasets in the Yangtze River Delta region, China.

Journal: Environmental pollution (Barking, Essex : 1987)
Published Date:

Abstract

Black carbon (BC) is a short-lived pollutant with significant environment and human health impacts. Monitoring BC is important, but its spatial coverage is limited. Therefore, predicting BC concentration is crucial in densely populated regions like the Yangtze River Delta (YRD). This study explores the machine learning (ML) models, including IAP, LASSO, RF, and SNN, to develop a robust BC prediction model for the YRD, based on BC behavior at the Dianshan Lake (DSL) site. The annual BC concentration at DSL was 1.37 μg/m, mainly from liquid fuel combustion (68 %), biomass burning (16 %), and coal combustion contributing (16 %). The ML model was first trained with DSL data (June 2021-June 2022) and then applied to other YRD sites in four scenarios based on air mass trajectories. The SNN model had R values over 0.80 for all scenarios at the DSL site. The model performed better during peak traffic periods, highlighting traffic's impact on BC levels. These models were applied to the YRD sites with R from 0.45 to 0.84. Hangzhou (HZ, 0.75-0.81), Nanjing (NJ, 0.78-0.80), and Pudong (PD, 0.76-0.84) showed the highest results. This suggests the model effectively captures BC concentrations from sources with similar emissions and meteorological conditions.

Authors

  • Lian Duan
    Department of Medical Informatics, Nantong University, Nantong, Jiangsu, China.
  • Pak Lun Fung
    Institute for Atmospheric and Earth System Research (INAR/Physics), Faculty of Science, University of Helsinki, PL 64, FI-00014, UHEL, Helsinki, Finland.
  • Qingyan Fu
    State Ecologic Environmental Scientific Observation and Research Station at Dianshan Lake, Shanghai Environmental Monitoring Center, Shanghai 200235, People's Republic of China.
  • Jia Chen
    Department of Oncology Internal Medicine, Nantong Tumor Hospital, Affiliated Tumor Hospital of Nantong University, Nantong, China.
  • Juntao Huo
    Shanghai Environmental Monitoring Center, Shanghai 200235, China.
  • Kan Huang
    Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, People's Republic of China.
  • Guochen Wang
    Key Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027, China.
  • Martha Arbayani Zaidan
    Institute for Atmospheric and Earth System Research (INAR/Physics), Faculty of Science, University of Helsinki, PL 64, FI-00014, UHEL, Helsinki, Finland; Department of Computer Science, Faculty of Science, University of Helsinki, PL 64, FI-00014, UHEL, Helsinki, Finland.
  • Zhigang Guo
    Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai, 200438, China; Institute of Eco-Chongming (IEC), Shanghai, 200062, China.
  • Tareq Hussein
    Institute for Atmospheric and Earth System Research (INAR/Physics), Faculty of Science, University of Helsinki, PL 64, FI-00014, UHEL, Helsinki, Finland; Environmental and Atmospheric Research Laboratory (EARL), Department of Physics, School of Science, University of Jordan, 11942, Amman, Jordan. Electronic address: tareq.hussein@helsinki.fi.