Predicting the higher heating value of syngas pyrolyzed from sewage sludge using an artificial neural network.

Journal: Environmental science and pollution research international
Published Date:

Abstract

Sludge pyrolysis is a complex process including complicated reaction chemistry, phase transition, and transportation phenomena. To better evaluate the use of syngas, the monitoring and prediction of a higher heating value (HHV) is necessary. This study developed an artificial neural network (ANN) model to predict the HHV of syngas, with the process variables (i.e., sludge type, catalyst type, catalyst amount, pyrolysis temperature, and moisture content) as the inputs. In the first step, through optimizing various sets of parameters, a three-layer network including 8 input neurons, 15 hidden neurons, and 1 output neuron was established. Then, in the second step, an ANN model has been successfully used to predict the HHV of syngas, with a fitting correlation coefficient of 0.97 and a root mean square error (MSE) value of 14.62. The relative influence of input variables showed that the pyrolysis temperature and moisture content were the determining factors that affected the HHV of syngas. The results of optimization experiments showed that when temperature was 895 °C and the moisture content was 45.63 wt%, the highest HHV can be obtained as 438.22 kcal/m-N. Moreover, the ANN model showed a higher prediction accuracy than other models like multiple linear regression and principal component regression. The model developed in this work may be used to predict the HHV of syngas using conventional operational parameters measured from in situ experiments, thus further providing predictive information for the use of syngas as energy and fuel.

Authors

  • Hongsen Li
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China.
  • Qi Xu
    State Key Lab of Urban and Regional Ecology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; Henan Institute of Advanced Technology, Zhengzhou University, Zhengzhou 450052, China.
  • Keke Xiao
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China. xiaokeke@mail.hust.edu.cn.
  • Jiakuan Yang
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China. jkyang@mail.hust.edu.cn.
  • Sha Liang
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China.
  • Jingping Hu
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China.
  • Huijie Hou
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China.
  • Bingchuan Liu
    School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, People's Republic of China.