Machine learning prediction and exploration of phosphorus migration and transformation during hydrothermal treatment of biomass waste.

Journal: The Science of the total environment
PMID:

Abstract

Hydrothermal treatment (HTT) held promise for phosphorus (P) recovery from high-moisture biomass. However, traditional experimental studies of P hydrothermal conversion were time-consuming and labor-intensive. Thus, based on biomass characteristics and HTT parameters, Random Forest (RF) and Gradient Boosting Regression machine learning (ML) models were constructed to predict HTT P migration between total P in hydrochar (TP_HC) and process water (TP_PW) and hydrochar P transformation among inorganic P (IP_HC), organic P (OP_HC), non-apatite inorganic P (NAIP_HC), and apatite P (AP_HC). Results demonstrated that the RF models (test R > 0.86) exhibited excellent performance in both single-target and multi-target predictions. Feature importance analysis identified TP_feed, O, C, and N as critical features influencing P distribution in hydrothermal products. TP_feed, NAIP_feed, temperature, and IP_feed were crucial factors affecting P form transformation in HC. This study provided valuable insights into understanding the migration and transformation of P and further guided experimental research.

Authors

  • Ying Tong
    School of Information and Communication Engineering, Nanjing Institute of Technology, Nanjing, 211167.
  • Weijin Zhang
    School of Energy Science and Engineering, Central South University, Changsha 410083, PR China.
  • Junhui Zhou
    School of Energy Science and Engineering, Central South University, Changsha 410083, China.
  • Shengqiang Liu
    Aerospace Kaitian Environmental Technology Co., Ltd., Changsha 410100, China.
  • Bingyan Kang
    School of Energy Science and Engineering, Central South University, Changsha 410083, China.
  • Jinghan Wang
    Department of Ophthalmology, Fudan Eye & ENT Hospital, Shanghai, China.
  • Shaojian Jiang
    School of Energy Science and Engineering, Central South University, Changsha 410083, China.
  • Lijian Leng
    School of Energy Science and Engineering, Central South University, Changsha 410083, China; Xiangjiang Laboratory, Changsha 410205, China. Electronic address: lljchs@126.com.
  • Hailong Li
    College of Energy, Xiamen University, Xiamen, 361005 People's Republic of China.