Machine learning-enhanced flavoromics: Identifying key aroma compounds and predicting sensory quality in sauce-flavor baijiu.

Journal: Food chemistry
PMID:

Abstract

The quality of Sauce-flavor baijiu hinges on sensory characteristics and key aroma compounds, which traditional methods struggle to evaluate accurately and effectively. This study explores the sensory characteristics and aroma compounds of Sauce-flavor baijiu across different rounds using flavoromics and machine learning, constructing quality grade prediction models. Sensory characteristics shift from acid in the early stages BJ1-BJ2 rounds to sauce in the mid-stages BJ3-BJ5 rounds and caramel in the late stages BJ6-BJ7 rounds. Employing AEDA and OAV analyses, 18 key odor-active compounds were identified, such as ethyl butyrate, ehyl isovalerate, and phenethyl acetate. Additionally machine learning models combined with clustering algorithms achieved high accuracy in predicting quality grades: 85 % (MLP+ HCA), 97 % (XGBoost+ K-means), and 84 % (Random Forest+ GMM). The SHAP model identified 20 key aroma compounds, including diethyl succinate, Tetramethylpyrazine, and Acetaldehyde, determining quality concentration thresholds. This study offers robust methods for baijiu flavor control and quality evaluation.

Authors

  • Shuai Li
    School of Molecular Biosciences, Center for Reproductive Biology, College of Veterinary Medicine, Washington State University.
  • Yueran Han
    Guizhou Guotai Digital-Intelligent Liquor Co., Ltd., Renhuai, Guizhou 564501, China.
  • Li Wang
    College of Marine Electrical Engineering, Dalian Maritime University, Dalian, China.
  • Ya Zhang
    Department of Plant Protection, College of Plant Protection, Hunan Agricultural University, Changsha, China. Electronic address: zhangya230@126.com.
  • Fan Wang
    Faculty of Information Engineering and Automation, Kunming University of Science and Technology, Kunming, China.
  • Youming Ou
    Guizhou Guotai Digital-Intelligent Liquor Co., Ltd., Renhuai, Guizhou 564501, China.
  • Haoying Li
    College of Liquor and Food Engineering, Key Laboratory of Fermentation Engineering and Biological Pharmacy of Guizhou Province, Guizhou University, Guiyang, Guizhou 550025, China; Key Laboratory of Fermentation Engineering and Biological Pharmacy of Guizhou Province, China.
  • Liang Yang
  • Shuyi Qiu
    College of Liquor and Food Engineering, Key Laboratory of Fermentation Engineering and Biological Pharmacy of Guizhou Province, Guizhou University, Guiyang, Guizhou 550025, China; Key Laboratory of Fermentation Engineering and Biological Pharmacy of Guizhou Province, China. Electronic address: syqiu@gzu.edu.cn.
  • Jun Lu
    School of Acupuncture-moxibustion and Tuina, Beijing University of Chinese Medicine, Beijing 100029, China.