Identification of Fusarium sambucinum species complex by surface-enhanced Raman spectroscopy and XGBoost algorithm.

Journal: Food chemistry
PMID:

Abstract

Rapid and reliable identification of Fusarium fungi is crucial, due to their role in food spoilage and potential toxicity. Traditional identification methods are often time-consuming and resource-intensive. This study explores the use of surface-enhanced Raman spectroscopy (SERS) to identify four species from the Fusarium sambucinum species complex isolated from barley. SERS spectra from 60 samples was acquired using gold nanoparticles for signal enhancement and the eXtreme Gradient Boosting (XGBoost) algorithm was applied for classification. The method achieved 100 % precision, recall, accuracy, and F1-score, thereby demonstrating excellent performance. Regarding the chemical interpretability, key spectral features at 495, 546, 764, 1228, 1274, and 1605 cm were revealed by XGBoost and correlated to the differences in chemical composition of fungi; particularly related to chitin, metabolites, and protein content. Therefore, SERS and XGBoost have great potential to classify a wide variety of fungi and other microorganisms.

Authors

  • Elem T S Caramês
    Department of Microbiology, Institute of Biomedical Sciences, University of São Paulo, 05508-900 São Paulo, Brazil.
  • Venancio F de Moraes-Neto
    Department of Food Science, School of Food Engineering, State University of Campinas, 13083-862 Campinas, São Paulo, Brazil.
  • Bruno G Bertozzi
    Department of Food Science, School of Food Engineering, State University of Campinas, 13083-862 Campinas, São Paulo, Brazil.
  • Leandro P da Silva
    Institute of Chemistry, State University of Campinas, 13083-970 Campinas, São Paulo, Brazil.
  • Javier E L Villa
    Instituto de Química, Universidade Estadual de Campinas (UNICAMP), Campinas, SP, 13083-970, Brazil. jelv@unicamp.br.
  • Juliana A L Pallone
    Department of Food Science, School of Food Engineering, State University of Campinas, 13083-862 Campinas, São Paulo, Brazil.
  • Liliana O Rocha
    Department of Food Science, School of Food Engineering, State University of Campinas, 13083-862 Campinas, São Paulo, Brazil.
  • Benedito Correa
    Department of Microbiology, Institute of Biomedical Sciences, University of São Paulo, 05508-900 São Paulo, Brazil. Electronic address: correabe@usp.br.