Engineering highly active nuclease enzymes with machine learning and high-throughput screening.

Journal: Cell systems
PMID:

Abstract

Optimizing enzymes to function in novel chemical environments is a central goal of synthetic biology, but optimization is often hindered by a rugged fitness landscape and costly experiments. In this work, we present TeleProt, a machine learning (ML) framework that blends evolutionary and experimental data to design diverse protein libraries, and employ it to improve the catalytic activity of a nuclease enzyme that degrades biofilms that accumulate on chronic wounds. After multiple rounds of high-throughput experiments, TeleProt found a significantly better top-performing enzyme than directed evolution (DE), had a better hit rate at finding diverse, high-activity variants, and was even able to design a high-performance initial library using no prior experimental data. We have released a dataset of 55,000 nuclease variants, one of the most extensive genotype-phenotype enzyme activity landscapes to date, to drive further progress in ML-guided design. A record of this paper's transparent peer review process is included in the supplemental information.

Authors

  • Neil Thomas
    Computer Science Division, University of California, Berkeley, Berkeley, CA 94720, USA.
  • David Belanger
    Google Brain, Cambridge, Massachusetts 02142, USA.
  • Chenling Xu
    Triplebar, Emeryville, CA 94608, USA.
  • Hanson Lee
    Triplebar, Emeryville, CA 94608, USA.
  • Kathleen Hirano
    Triplebar, Emeryville, CA 94608, USA.
  • Kosuke Iwai
    Triplebar, Emeryville, CA 94608, USA.
  • Vanja Polic
    Triplebar, Emeryville, CA 94608, USA.
  • Kendra D Nyberg
    Triplebar, Emeryville, CA 94608, USA.
  • Kevin G Hoff
    Triplebar, Emeryville, CA 94608, USA.
  • Lucas Frenz
    Triplebar, Emeryville, CA 94608, USA.
  • Charlie A Emrich
    X, the Moonshot Factory, Mountain View, CA 94043, USA.
  • Jun W Kim
    X, the Moonshot Factory, Mountain View, CA 94043, USA.
  • Mariya Chavarha
    Google Accelerated Sciences, Mountain View, CA 94043, USA.
  • Abi Ramanan
    X, the Moonshot Factory, Mountain View, CA 94043, USA.
  • Jeremy J Agresti
    Triplebar, Emeryville, CA 94608, USA.
  • Lucy J Colwell
    Department of Chemistry, Cambridge University, Cambridge, UK. Electronic address: ljc37@cam.ac.uk.