Image learning to accurately identify complex mixture components.

Journal: The Analyst
Published Date:

Abstract

The study of complex mixtures is very important for exploring the evolution of natural phenomena, but the complexity of the mixtures greatly increases the difficulty of material information extraction. Image perception-based machine-learning techniques have the ability to cope with this problem in a data-driven way. Herein, we report a 2D-spectral imaging method to collect matter information from mixture components, and the obtained feature images can be easily provided to deep convolutional neural networks (CNNs) for establishing a spectral network. The results demonstrated that a single CNN trained end-to-end from the proposed images can directly accomplish synchronous measurement of multi-component samples using only raw pixels as inputs. Our strategy has some innate advantages, such as fast data acquisition, low cost, and simple chemical treatment, suggesting that it can be extensively applied in many fields, including environmental science, biology, medicine, and chemistry.

Authors

  • Qiannan Duan
    State Key Laboratory of Pollution Control and Resource Reuse, Jiangsu Key Laboratory of Vehicle Emissions Control, School of the Environment, Nanjing University, Nanjing 210023, China.
  • Jianchao Lee
    Department of Environment Science, Shaanxi Normal University, Xi'an 710062, China.
  • Jiayuan Chen
    Department of Environment Science, Shaanxi Normal University, Xi'an 710062, China.
  • Yunjin Feng
    Department of Environmental Science, Shaanxi Normal University, Xi'an 710062, China. jianchaolee@snnu.edu.cn.
  • Run Luo
    Department of Environmental Science, Shaanxi Normal University, Xi'an 710062, China. jianchaolee@snnu.edu.cn.
  • Can Wang
    School of Acu-Mox and Tuina, Chengdu University of Traditional Chinese Medicine, Chengdu, China.
  • Sifan Bi
    Department of Environment Science, Shaanxi Normal University, Xi'an 710062, China.
  • Fenli Liu
    Department of Environmental Science, Shaanxi Normal University, Xi'an 710062, China. jianchaolee@snnu.edu.cn.
  • Wenjing Wang
    School of Economics, Tianjin University of Commerce, Tianjin, 300134, China. Electronic address: maggiewwj@163.com.
  • Yicai Huang
    Department of Environmental Science, Shaanxi Normal University, Xi'an 710062, China. jianchaolee@snnu.edu.cn.
  • Zhaoyi Xu
    State Key Laboratory of Pollution Control and Resource Reuse, Jiangsu Key Laboratory of Vehicle Emissions Control, School of the Environment, Nanjing University, Nanjing 210023, China. Electronic address: zhaoyixu@nju.edu.cn.