Investigation of spatiotemporal distribution and formation mechanisms of ozone pollution in eastern Chinese cities applying convolutional neural network.

Journal: Journal of environmental sciences (China)
PMID:

Abstract

Severe ground-level ozone (O) pollution over major Chinese cities has become one of the most challenging problems, which have deleterious effects on human health and the sustainability of society. This study explored the spatiotemporal distribution characteristics of ground-level O and its precursors based on conventional pollutant and meteorological monitoring data in Zhejiang Province from 2016 to 2021. Then, a high-performance convolutional neural network (CNN) model was established by expanding the moment and the concentration variations to general factors. Finally, the response mechanism of O to the variation with crucial influencing factors is explored by controlling variables and interpolating target variables. The results indicated that the annual average MDA8-90 concentrations in Zhejiang Province are higher in the northern and lower in the southern. When the wind direction (WD) ranges from east to southwest and the wind speed (WS) ranges between 2 and 3 m/sec, higher O concentration prone to occur. At different temperatures (T), the O concentration showed a trend of first increasing and subsequently decreasing with increasing NO concentration, peaks at the NO concentration around 0.02 mg/m. The sensitivity of NO to O formation is not easily affected by temperature, barometric pressure and dew point temperature. Additionally, there is a minimum [Formula: see text] at each temperature when the NO concentration is 0.03 mg/m, and this minimum [Formula: see text] decreases with increasing temperature. The study explores the response mechanism of O with the change of driving variables, which can provide a scientific foundation and methodological support for the targeted management of O pollution.

Authors

  • Qiaoli Wang
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Dongping Sheng
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Chengzhi Wu
    Trinity Consultants, Inc. (China office), Hangzhou 310012, China.
  • Xiaojie Ou
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Shengdong Yao
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Jingkai Zhao
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Feili Li
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China.
  • Wei Li
    Department of Nephrology, The Second Affiliated Hospital of Guangxi Medical University, Nanning, Guangxi, China.
  • Jianmeng Chen
    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China; Zhejiang University of Science & Technology, Hangzhou 310023, China. Electronic address: jchen@zjut.edu.cn.