Chemiresistive Sensor Array and Machine Learning Classification of Food.

Journal: ACS sensors
Published Date:

Abstract

Successful identification of complex odors by sensor arrays remains a challenging problem. Herein, we report robust, category-specific multiclass-time series classification using an array of 20 carbon nanotube-based chemical sensors. We differentiate between samples of cheese, liquor, and edible oil based on their odor. In a two-stage machine-learning approach, we first obtain an optimal subset of sensors specific to each category and then validate this subset using an independent and expanded data set. We determined the optimal selectors via independent selector classification accuracy, as well as a combinatorial scan of all 4845 possible four selector combinations. We performed sample classification using two models-a -nearest neighbors model and a random forest model trained on extracted features. This protocol led to high classification accuracy in the independent test sets for five cheese and five liquor samples (accuracies of 91% and 78%, respectively) and only a slightly lower (73%) accuracy on a five edible oil data set.

Authors

  • Vera Schroeder
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.
  • Ethan D Evans
    Department of Biological Engineering , Massachusetts Institute of Technology , Cambridge Massachusetts 02139 , United States.
  • You-Chi Mason Wu
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.
  • Constantin-Christian A Voll
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.
  • Benjamin R McDonald
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.
  • Suchol Savagatrup
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.
  • Timothy M Swager
    Department of Chemistry and Institute for Soldier Nanotechnologies , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge Massachusetts 02139 , United States.