Biosynthesis of copper nanoparticles using Shewanella loihica PV-4 with antibacterial activity: Novel approach and mechanisms investigation.

Journal: Journal of hazardous materials
PMID:

Abstract

Metallic nanoparticle based disinfection represents a promising approach for microbial pollution control in drinking water and thus, biosynthesis of non precious metal nanoparticles is of considerable interest. Herein, an original and efficient route for directly microbial synthesis of copper nanoparticles (Cu-NPs) by Shewanella loihica PV-4 is described and their satisfactorily antimicrobial activities are established. Cu-NPs were successfully synthesized and most of them attaching on the bacterial cell surfaces suggested extracellular Cu(II) bioreduction mainly contributed to this biosynthesis. Using a suite of characterization methods, polycrystalline nature and face centered cubic lattice of Cu-NPs were revealed, with size in the range of 10-16 nm. With Cu-NPs dosage of 100 μg/mL and 10 CFU/mL fresh Escherichia coli suspension, the obtained antibacterial efficiency reached as high as 86.3 ± 0.2% within 12 h. Cell damages were primarily caused by the generated reactive oxygen species with HO playing significant roles. Both cell membrane and cytoplasm components were destroyed, while the key inactivation mechanisms were lipid peroxidation and DNA damage as concluded through correlation analysis. The cost-effective and eco-friendly biosynthesis of Cu-NPs with high antibacterial activities make them particularly attractive for drinking water disinfection.

Authors

  • Qing Lv
    School of Water Resources and Environment, MOE Key Laboratory of Groundwater Circulation and Environmental Evolution, China University of Geosciences (Beijing), Beijing 100083, PR China.
  • Baogang Zhang
    School of Water Resources and Environment, MOE Key Laboratory of Groundwater Circulation and Environmental Evolution, China University of Geosciences (Beijing), Beijing 100083, PR China. Electronic address: zbgcugb@gmail.com.
  • Xuan Xing
    College of Life and Environmental Science, Minzu University of China, Beijing 100081, PR China.
  • Yingxin Zhao
    School of Environmental Science and Engineering, Tianjin University, Tianjin 300350, PR China.
  • Ruquan Cai
    School of Water Resources and Environment, MOE Key Laboratory of Groundwater Circulation and Environmental Evolution, China University of Geosciences (Beijing), Beijing 100083, PR China.
  • Wei Wang
    State Key Laboratory of Quality Research in Chinese Medicine, Institute of Chinese Medical Sciences, University of Macau, Macau 999078, China.
  • Qian Gu
    School of Water Resources and Environment, MOE Key Laboratory of Groundwater Circulation and Environmental Evolution, China University of Geosciences (Beijing), Beijing 100083, PR China.