Chemical characterization and wound healing property of a β-D-glucan from edible mushroom Piptoporus betulinus.

Journal: International journal of biological macromolecules
PMID:

Abstract

A water-soluble β-D-glucan was obtained from fruiting bodies of Piptoporus betulinus, by hot aqueous extraction followed by freeze-thawing procedure and dialysis. Its molar mass distribution and conformational behavior in solution was assessed by size-exclusion chromatography coupled with multiangle laser light scattering, showing a polysaccharide with an average molecular weight of 2.5 × 10 Da with a random coil conformation for molecular weights below 1 × 10 Da. Typical signals of β-(1 → 3)-linkages were observed in NMR spectrum (δ 102.7/4.76; 102.8/4.74; 102.9/4.52; and δ 85.1/3.78; 85.0/3.77) and also signals of O-6 substitution at δ 69.2/4.22 and 69.2/3.87. The analysis of partially O-methylated alditol acetates corroborates the NMR results, indicating the presence of a β-D-glucan with a main chain (1 → 3)-linked, substituted at O-6 by single-units of glucose. The β-D-glucan showed no toxicity on human colon carcinoma cell line (Caco-2) up to 1000 μg mL and promoted cell migration on in vitro scratch assay, demonstrating a potential wound healing capacity.

Authors

  • Liana Inara de Jesus
    Department of Biochemistry and Molecular Biology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil.
  • Fhernanda R Smiderle
    Department of Biochemistry and Molecular Biology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil.
  • Andrea C Ruthes
    Division of Glycoscience, AlbaNova University Centre, Royal Institute of Technology, 106 91 Stockholm, Sweden.
  • Francisco Vilaplana
    Division of Glycoscience, AlbaNova University Centre, Royal Institute of Technology, 106 91 Stockholm, Sweden.
  • Fernando Tonholi Dal'Lin
    Department of Pharmacology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil.
  • Daniele Maria-Ferreira
    Department of Biochemistry and Molecular Biology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil; Department of Pharmacology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil.
  • Maria Fernanda Werner
    Department of Pharmacology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil.
  • Leo J L D Van Griensven
    Plant Research International, Wageningen University and Research, Bornsesteeg 1, 6708 PD Wageningen, The Netherlands.
  • Marcello Iacomini
    Department of Biochemistry and Molecular Biology, Federal University of Parana, CP 19046, Curitiba, PR, Brazil. Electronic address: iacomini@ufpr.br.