Cytotoxicity of the Defensive Secretion from the Medicinal Insect Blaps rynchopetera.

Journal: Molecules (Basel, Switzerland)
Published Date:

Abstract

Fairmaire has long been used as a folk medicine by the Yi and Bai ethnic groups in China to treat fever, cough, gastritis, boils, and tumors. In the present study, the cytotoxicity of the defensive secretion (TDS) of against AGS Caco-2, HepG2 U251 and Bel-7402 was tested, and the results revealed that TDS had potent cytotoxicity against testing cells with IC values of 45.8, 17.4, 53.6, 98.4 and 23.4 μg/mL, respectively. Gas chromatography-mass spectrometry (GC-MS) analysis was employed to clarify the cytotoxic constituents in TDS of and five volatile compounds, including 2-ethyl-2,5-cyclohexadiene-1,4-dione (, 31.00%), 1-tridecene (, 28.02%), 2-methyl-2,5-cyclohexadiene-1,4-dione (, 22.86%), hydroquinone (, 1.33%), and -benzoquinone (, 1.01%), were identified. Chemical constituent investigation on TDS further supported the presence of 5 above compounds. A cytotoxic assay indicated that compounds , , and exhibited significant cytotoxicity against the testing cell lines, implying that benzoquinones and hydroquinone played important roles in the cytotoxicity of TDS of . TDS is a cytotoxic natural material and further studies investigating mechanisms and inhibitory activities on other cell lines is warranted.

Authors

  • Huai Xiao
    Functional Molecules Analysis and Biotransformation Key Laboratory of Universities in Yunnan Province, School of Chemical Science and Technology, Yunnan University, Kunming 650091, China. Xiaohuai10@263.net.
  • Jian-Wei Dong
    Functional Molecules Analysis and Biotransformation Key Laboratory of Universities in Yunnan Province, School of Chemical Science and Technology, Yunnan University, Kunming 650091, China.
  • Di-Jiao Zhou
    Functional Molecules Analysis and Biotransformation Key Laboratory of Universities in Yunnan Province, School of Chemical Science and Technology, Yunnan University, Kunming 650091, China. jwdongyn@outlook.com.
  • Xiu-Mei Wu
    Yunnan Provincial Key Laboratory of Entomological Biopharmaceutical R&D, Dali University, Dali 671000, China. 13648847405@163.com.
  • Jian-Rong Luo
    Yunnan Provincial Key Laboratory of Entomological Biopharmaceutical R&D, Dali University, Dali 671000, China. caile@ynu.edu.cn.
  • Cheng-Gui Zhang
    Yunnan Provincial Key Laboratory of Entomological Biopharmaceutical R&D, Dali University, Dali 671000, China. wxm6865@163.com.
  • Na-Na Guo
    Yunnan Provincial Key Laboratory of Entomological Biopharmaceutical R&D, Dali University, Dali 671000, China. ljrrong@vip.sina.com.
  • Yue Li
    School of Computer Science and Software Engineering, University of Science and Technology Liaoning, Anshan, China.
  • Le Cai
    Functional Molecules Analysis and Biotransformation Key Laboratory of Universities in Yunnan Province, School of Chemical Science and Technology, Yunnan University, Kunming 650091, China. chenggui_zcg@163.com.
  • Zhong-Tao Ding
    Functional Molecules Analysis and Biotransformation Key Laboratory of Universities in Yunnan Province, School of Chemical Science and Technology, Yunnan University, Kunming 650091, China. ztding@ynu.edu.cn.