Deep-Learning-Assisted Microfluidic Immunoassay via Smartphone-Based Imaging Transcoding System for On-Site and Multiplexed Biosensing.

Journal: Nano letters
PMID:

Abstract

Point-of-care testing (POCT) with multiplexed capability, ultrahigh sensitivity, affordable smart devices, and user-friendly operation is critically needed for clinical diagnostics and food safety. This study presents a deep-learning-assisted microfluidic immunoassay platform that uses a smartphone-based imaging transcoding system, polystyrene microsphere-based encoding, and artificial-intelligence-assisted decoding. Microspheres of varying sizes act as multiprobes, with their quantities correlating to target concentrations after an immunoreaction and separation-filtration within the microfluidic chip. A smartphone with intelligent decoding software captures images of multiprobes from the chip and performs classification, counting, and concentration calculations. The "encoding-decoding" strategy and integrated microfluidic chip design allow these processes to be completed in simple steps, eliminating the need for additional immunomagnetic separation. As a proof of concept, this platform successfully detected multiple respiratory viruses and antibiotics in various real samples with high sensitivity within 30 min, demonstrating great potential as a smart, universal toolkit for next-generation POCT applications.

Authors

  • Peng Lu
    Department of Industrial Design, Dalian University of Technology, Dalian 116024, China.
  • Yang Zhou
    State Environmental Protection Key Laboratory of Environmental Pollution Health Risk Assessment, South China Institute of Environmental Sciences, Ministry of Environmental Protection, Guangzhou, China.
  • Xiaohu Niu
    College of Engineering, Huazhong Agricultural University, Wuhan 430070, Hubei, China.
  • Chen Zhan
    College of Engineering, Huazhong Agricultural University, Wuhan 430070, China.
  • Pengzhou Lang
    Henan Mechanical & Electrical Vocational College, Zhengzhou 451192, China.
  • Yongkun Zhao
    College of Food Science and Technology, Huazhong Agricultural University, Wuhan, 430070, Hubei China.
  • Yiping Chen
    Beijing Engineering Research Center for BioNanotechnology & CAS Key Laboratory for Biological Effects of Nanomaterials and Nanosafety, National Center for Nanoscience and Technology, Beijing 100190, PR China. Electronic address: chenyp@nanoctr.cn.