Fluorescent sensor array for rapid bacterial identification using antimicrobial peptide-functionalized gold nanoclusters and machine learning.

Journal: Talanta
PMID:

Abstract

Bacterial infectious diseases pose significant challenges to public health, emphasizing the need for rapid and accurate diagnostic tools. Here, we introduced a multichannel fluorescent sensor array based on antimicrobial peptide-functionalized gold nanoclusters (AMP-AuNCs) designed for precise bacterial identification. By utilizing the unique electrostatic and hydrophobic properties of three AMP-AuNCs, this sensor array generated distinct fluorescence patterns upon binding to different bacterial species. Machine learning algorithms, including Principal Component Analysis (PCA), Hierarchical Clustering Analysis (HCA), and Linear Discriminant Analysis (LDA), were employed to analyze fluorescence fingerprint patterns and identify bacterial strains with high accuracy. The sensor array achieved 100 % accuracy in identifying six common bacterial species and demonstrated an 86.7 % accuracy in classifying clinical Escherichia coli isolates from urinary tract infections. This AMP-AuNC-based sensor array offers a promising approach for rapid and precise bacterial diagnostics, with potential applications in clinical settings for combating antibiotic resistance.

Authors

  • Renjie Liu
    Zhengzhou Research Institute, Harbin Instituteof Technology, 150000, Nangang District, Xidazhi Street No. 90, Harbin, Heilongjiang, China.
  • Pengcheng Wang
    Department of Plant Protection, Henan Institute of Science and Technology, Xinxiang, China.
  • Yiliang Chen
    School of Nursing, The Hong Kong Polytechnic University, Hong Kong, China.
  • Fuyuan Huang
    Wenzhou Key Laboratory of Sanitary Microbiology, Key Laboratory of Laboratory Medicine, Ministry of Education, School of Laboratory Medicine and Life Sciences, Wenzhou Medical University, Wenzhou, 325035, China.
  • Yunqiu Shen
    Jiaxing University Affiliated TCM Hospital, Jiaxing, 314000, China. Electronic address: 17853735882@163.com.
  • Yan Zheng
    School of Computer Science, Northwestern Polytechnical University, West Youyi Road 127, Xi'an, 710072, China.
  • Laibao Zheng
    Wenzhou Key Laboratory of Sanitary Microbiology, Key Laboratory of Laboratory Medicine, Ministry of Education, School of Laboratory Medicine and Life Sciences, Wenzhou Medical University, Wenzhou, 325035, China. Electronic address: zhenglaibao@wmu.edu.cn.