Label-free multiplexed microtomography of endogenous subcellular dynamics using generalizable deep learning.

Journal: Nature cell biology
PMID:

Abstract

Simultaneous imaging of various facets of intact biological systems across multiple spatiotemporal scales is a long-standing goal in biology and medicine, for which progress is hindered by limits of conventional imaging modalities. Here we propose using the refractive index (RI), an intrinsic quantity governing light-matter interaction, as a means for such measurement. We show that major endogenous subcellular structures, which are conventionally accessed via exogenous fluorescence labelling, are encoded in three-dimensional (3D) RI tomograms. We decode this information in a data-driven manner, with a deep learning-based model that infers multiple 3D fluorescence tomograms from RI measurements of the corresponding subcellular targets, thereby achieving multiplexed microtomography. This approach, called RI2FL for refractive index to fluorescence, inherits the advantages of both high-specificity fluorescence imaging and label-free RI imaging. Importantly, full 3D modelling of absolute and unbiased RI improves generalization, such that the approach is applicable to a broad range of new samples without retraining to facilitate immediate applicability. The performance, reliability and scalability of this technology are extensively characterized, and its various applications within single-cell profiling at unprecedented scales (which can generate new experimentally testable hypotheses) are demonstrated.

Authors

  • YoungJu Jo
    Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Daejeon, 34141, Republic of Korea.
  • Hyungjoo Cho
    Department of Cardiology, University of Ulsan College of Medicine, Asan Medical Center, Seoul, Korea.
  • Wei Sun Park
    Department of Physics, Korea Advanced Institute of Science and Technology; KAIST Institute for Health Science and Technology, Korea Advanced Institute of Science and Technology.
  • Geon Kim
    Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Daejeon, Republic of Korea.
  • DongHun Ryu
  • Young Seo Kim
    Department of Neurology, College of Medicine, Hanyang University Seoul Hospital, Seoul, Republic of Korea.
  • Moosung Lee
    Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Daejeon, Republic of Korea.
  • Sangwoo Park
    Department of Animal Science, University of California, Davis, CA 95616, USA.
  • Mahn Jae Lee
    KAIST Institute for Health Science and Technology, KAIST, Daejeon, Republic of Korea.
  • Hosung Joo
    School of Electrical Engineering, KAIST, Daejeon 34141, Republic of Korea.
  • HangHun Jo
    Tomocube, Daejeon, Republic of Korea.
  • Seongsoo Lee
    Gwangju Center , Korea Basic Science Institute (KBSI) , Gwangju , 61186 , Korea.
  • Sumin Lee
    Tomocube, Inc.
  • Hyun-Seok Min
    1 Department of Cardiology University of Ulsan College of Medicine Asan Medical Center Seoul Korea.
  • Won Do Heo
    Department of Biological Sciences, KAIST, Daejeon, Republic of Korea. wdheo@kaist.ac.kr.
  • YongKeun Park
    Department of Physics, Korea Advanced Institute of Science and Technology (KAIST), Daejeon, 34141, Republic of Korea. yk.park@kaist.ac.kr.